厦门大学化学化工学院谢顺吉

paoshan

谢顺吉，厦门大学教授。2008和2011年于湖南大学获学士和硕士学位；2014年于厦门大学获博士学位；2014-2018年厦门大学能源材料化学协同创新中心iChEM博士后和研究员（合作导师：王野教授、李灿院士）。2019年获“中国催化新秀奖”，2020年获“国家优秀青年科学基金”资助。主要研究领域为C1分子和生物质的光催化和电催化选择转化，包括：CO2还原、乙二醇合成、甲烷氧化和生物质高值化利用。在Nature Catal., Nature Commun., Energy Environ. Sci., Chem, Angew. Chem. Int. Ed., Adv. Mater., ACS Catal.等国际学术刊物上发表论文30余篇。


谢顺吉
Email: shunji_xie@xmu.edu.cn


个人简历：
Education
Ph.D. in Physical Chemistry                               Xiamen University     Sep 2011 – Sep 2014
M.S. in Chemical Engineering & Technology      Hunan University      Sep 2008 – Jul 2011
B.S. in Chemical Engineering & Technology       Hunan University     Sep 2004 – Jul 2008


Employment
Senior Engineer, State Key Laboratory of Physical Chemistry of Solid Surfaces, Xiamen University
Jun 2018 – Present
iChEM Research Fellow, Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)
Sep 2017 – May 2018
iChEM Postdoc, Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)
Sep 2014 – Sep 2017
Award
China Catalysis Award for Rising Star (中国催化新秀奖)     Jul 2019
ACS Catalysis Award for Early Career Researcher             Jul 2018


Project & Funding
National Natural Science Foundation of China, 2016-2018.
ŸFirst-class General Financial Grant from the China Postdoctoral Science Foundation, 2015-2017.
Special Financial Grant from the China Postdoctoral Science Foundation, 2016-2017.


研究兴趣：
Photocatalysis and electrocatalysis for CO2 reduction, biomass conversion, ethylene glycol synthesis and methane selective conversion.


近期主要代表论著：
[1]      Wenchao Ma, Shunji Xie(co-first author), Xia-Guang Zhang, Fanfei Sun, Jincan Kang, Zheng Jiang, Qinghong Zhang,* De-Yin Wu,* Ye Wang,* Promoting electrocatalytic CO2 reduction to formate via sulfur-boosting water activation on indium surfaces, Nature Commun., 2019, 10, 892.
[2]      Longfu Wei, Jinchi Lin, Shunji Xie,* Wenchao Ma, Qinghong Zhang, Zebin Shen, Ye Wang,* Photoelectrocatalytic reduction of CO2 to syngas over Ag nanoparticle modified p-Si nanowire arrays, Nanoscale, 2019, 11, 12530-12536 (Outside Back Cover).
[3]      Xuejiao Wu, Shunji Xie(co-first author), Chenxi Liu, Cheng Zhou, Jinchi Lin, Jincan Kang, Qinghong Zhang,* Zhaohui Wang,* Ye Wang,* Ligand-Controlled Photocatalysis of CdS Quantum Dots for Lignin Valorization under Visible Light, ACS Catal., 2019, accepted.
[4]      Shunji Xie, Ye Wang,* Recent Advances, Challenges and Perspectives in Selective Oxidation Catalysis, Chin. J. Catal., 2019, accepted. (Special Issue for NSFC, 催化与表界面化学学科前沿与发展战略研讨会特刊)
[5]      Shunji Xie, Zebin Shen, Jiao Deng, Pu Guo, Qinghong Zhang, Haikun Zhang, Chao Ma, Zheng Jiang, Jun Cheng,* Dehui Deng,* Ye Wang,* Visible light-driven C−H activation and C–C coupling of methanol into ethylene glycol, Nature Commun., 2018, 9, 1181.
[6]      Xuejiao Wu, Xueting Fan, Shunji Xie(co-first author), Jinchi Lin, Jun Cheng,* Qinghong Zhang,*  Liangyi Chen, Ye Wang,* Solar energy-driven lignin-first approach to full utilization of lignocellulosic biomass under mild conditions, Nature Catal., 2018, 1, 772-780.
[7]      Shunji Xie,* Shengqi Lin, Qinghong Zhang,* Zhongqun Tian, Ye Wang, Selective electrocatalytic conversion of methane to fuels and chemicals, J. Energy Chem., 2018, 27, 1629-1636.
[8]      Shunji Xie, Zebin Shen, Huamin Zhang, Jun Cheng, Qinghong Zhang,* Ye Wang,* Photocatalytic coupling of formaldehyde to ethylene glycol and glycolaldehyde over bismuth vanadate with controllable facets and cocatalysts, Catal. Sci. Technol., 2017, 7, 923-933.
[9]      Shunji Xie, Qinghong Zhang,* Guodong Liu, Ye Wang,* Photocatalytic and photoelectrocatalytic reduction of CO2 using heterogeneous catalysts with controlled nanostructures, Chem. Commun., 2016, 52, 35-59.
[10]  Zebin Shen, Shunji Xie(co-first author), Wenqing Fan, Qinghong Zhang,* Zaiku Xie, Weimin Yang, Yangdong Wang, Jinchi Lin, Xuejiao Wu, Huilin Wana, Ye Wang,* Direct conversion of formaldehyde to ethylene glycol via photocatalytic carbon-carbon coupling over bismuth vanadate, Catal. Sci. Technol., 2016, 6, 6485-6489.
[11]  Shunji Xie, Yu Wang, Qinghong Zhang,* Weiping Deng, Ye Wang,* SrNb2O6 nanoplates as efficient photocatalysts for the preferential reduction of CO2 in the presence of H2O, Chem. Commun., 2015, 51, 3430-3433.
[12]  Guodong Liu, Shunji Xie(co-first author), Qinghong Zhang,* Zhengfang Tian, Ye Wang,* Carbon dioxide-enhanced photosynthesis of methane and hydrogen from carbon dioxide and water over Pt-promoted polyaniline-TiO2 nanocomposites, Chem. Commun., 2015, 51, 13654-13657.
[13]  Shunji Xie, Yu Wang, Qinghong Zhang,* Weiping Deng, Ye Wang,* MgO- and Pt-Promoted TiO2 as an Efficient Photocatalyst for the Preferential Reduction of Carbon Dioxide in the Presence of Water, ACS Catal., 2014, 4, 3644-3653.
[14]  Qingge Zhai, Shunji Xie(co-first author), Wenqing Fan, Qinghong Zhang,* Yu Wang, Weiping Deng, Ye Wang,* Photocatalytic conversion of carbon dioxide with water into methane: platinum and copper (I) oxide co-catalysts with a core-shell structure, Angew. Chem. Int. Ed., 2013, 52, 5776-5779.
[15]  Shunji Xie, Yu Wang, Qinghong Zhang,* Wenqing Fan, Weiping Deng, Ye Wang,* Photocatalytic reduction of CO2 with H2O: significant enhancement of the activity of Pt-TiO2 in CH4 formation by addition of MgO, Chem. Commun., 2013, 49, 2451-2453.
[16]  Longfu Wei, Junxian Zhang, Weiping Deng,* Shunji Xie, Qinghong Zhang,* Ye Wang,* Catalytic transformation of 2,5-furandicarboxylic acid to adipic acid over niobic acid-supported Pt nanoparticles, Chem. Commun., 2019, 55, 8013-8016.
[17]  Quan Quan, Shunji Xie, Bo Weng, Nan Zhang, Ye Wang,* Yi-Jun Xu,* Revealing the Double-Edged Sword Role of Graphene on Boosted Charge Transfer versus Active Site Control in TiO2 Nanotube Arrays@RGO/MoS2Heterostructure, Small, 2018, 1704531.
[18]  Quan Quan, Shunji Xie, Ye Wang,* Yi-Jun Xu,* Photoelectrochemical Reduction of CO2 over Graphene-Based Composites: Basic Principle, Recent Progress, and Future Perspective, Acta Phys. -Chim. Sin., 2017, 33, 2404-2423.
[19]  Hao Yin, Jun Yi, Zhen-Wei Yang, Zhen-Yang Xu, Shunji Xie, Lei Li, Chao-Yu Li, Juan Xu, Hua Zhang,* San-Jun Zhang, Jian-Feng Li,* Zhong-Qun Tian. Plasmon enhanced quantum dots fluorescence and energy conversion in water splitting using shell-isolated nanoparticles, Nano Energy, 2017, 42, 232-240.
[20]  Nan Zhang, Shunji Xie, Bo Weng, Yi-Jun Xu,* Vertically aligned ZnO-Au@CdS core-shell nanorod arrays as an all-solid-state vectorial Z-scheme system for photocatalytic application, J. Mater. Chem. A, 2016, 4, 18804-18814.
[21]  Rui shen, Fei Yang, Jianping Wang, Yong Li, Shunji Xie, Chunyan Chen, Qingyun Cai,* Shouzhuo Yao, Application of magnetic material in the determination of polycyclic aromatic hydrocarbons in tree leaves by high performance liquid chromatography, Anal. Methods, 2011, 3, 2909-2914.
[22]  Dalei Sun, Shunji Xie, Jianru Deng, Caijuan Huang, Eli Ruckenstein,* Zisheng Chao,* CH3COONa as an effective catalyst for methoxycarbonylation of 1,6-hexanediamine by dimethyl carbonate to dimethylhexane-1,6-dicarbamate, Green Chem., 2010, 12, 483-490.

paoshan

甲醇直接脱氢偶联制乙二醇研究
批准号        21972115       
学科分类        多相催化 ( B020103 )
项目负责人        谢顺吉       
依托单位        厦门大学
资助金额        65.00万元       
项目类别        面上项目       
研究期限        2020 年 01 月 01 日 至2023 年 12 月 31 日

haoyou

近日，我院王野教授、谢顺吉教授研究团队与比利时鲁汶大学Bert Sels教授课题组合作撰写的综述性论文“Metal Sulfide Photocatalysts for Lignocellulose Valorization”发表于Advanced Materials (DOI: 10.1002/adma.202007129)。该篇综述为庆祝厦门大学百年校庆专刊论文之一。
       木质纤维素是最主要的可再生碳资源，将其转化成碳基化学品和液体燃料是生物质转化利用的理想途径之一。光催化已成为温和条件下生物质高效高选择性转化利用的新兴方法。C−O、C−C键的选择性裁剪和特定官能团的定向活化是光催化木质纤维素转化的关键挑战。近年来，已有研究发现金属硫化物半导体可实现高效光催化C−H键活化、C−O键切断、C−C偶联、选择性氧化等生物质选择性转化中具有挑战性的反应过程。金属硫化物在光催化木质纤维素选择转化中取得了重要进展，包括：木质纤维素解聚制平台分子；平台分子转化制醛、酸、高碳化合物、二元醇及氨基酸等。本综述对近期金属硫化物光催化木质纤维素选择转化的重要研究进展进行了系统总结与梳理，从材料性质角度解析了金属硫化物在木质纤维素转化过程中的优势，详细介绍了金属硫化物在特定光催化木质纤维素转化反应中的应用。综述重点讨论了金属硫化物在光催化木质纤维素相关平台分子选择转化中的催化机理，对金属硫化物性质及其在生物质转化反应过程中的独特作用进行分析，为高效高选择性的光催化剂设计提供借鉴，并对金属硫化物在光催化木质纤维素转化领域中的挑战和机遇进行了系统总结和展望。

       王野教授团队一直致力于生物质及其平台分子选择性催化转化方向的研究，发展了一系列生物质转化利用的新路线和高效催化体系(Angew. Chem. Int. Ed. 2021, 60, 4712; Chem 2020, 11, 3038; Chem. Soc. Rev. 2020, 49, 6198; ACS. Catal. 2019, 9, 8443; Nat. Catal. 2018, 1, 772; PNAS 2018, 115, 5093; Nat. Commun. 2013, 4, 2141)。
        该论文第一作者为我院2015级博士生吴雪娇(现为比利时鲁汶大学博士后)，我院王野教授、谢顺吉教授和比利时鲁汶大学Bert Sels教授为共同通讯作者。论文中相关研究工作得到国家自然科学基金(21690082、21972115、22022201)，鲁汶大学博士后基金(PDM/20/117)等项目的资助。
        论文链接：https://onlinelibrary.wiley.com/doi/full/10.1002/adma.202007129