青岛科技大学材料学院袁勋

xirui · 发表于 2017-10-12 09:06:36

袁勋，博士，青岛科技大学教授。2006和2009年在山东理工大学分别获得学士和硕士学位；2014年在新加坡国立大学获得博士学位。2014年2月起加入新加坡科技局辖属的生物工程与纳米技术研究所从事博士后研究，于2017年4月晋升为研究科学家。2017年8月入选青岛科技大学“第四人才层次”，加入青岛科技大学材料科学与工程学院, 任教授PI。

姓名  袁勋
性别  男
出生年月 1984年5月
职称教授
学历（学位）博士研究生（哲学博士）
毕业院校新加坡国立大学
所属院系  材料科学与工程学院
行政职务
导师类别  硕士生导师
主讲课程
招生专业  材料化学、应用化学、材料物理、新能源材料与器件
研究方向  金属纳米团簇，无机纳米材料，催化，生物医学
联系方式  yuanxun@qust.edu.cn; 电话: 13789870350; QQ: 108410224
办公室/实验室  CCE大楼1308室
个人简历 (包括近期科研项目)
个人简历：
袁勋近五年的研究工作集中于超小金属纳米团簇（<2纳米）的设计，合成及应用，通过对团簇尺寸、荧光特性，表面特性、组成和结构等的精确调控，实现其在生物分子及重金属离子检测、广谱抗菌、光热治疗、催化等领域的应用。因其博士期间出色的学术表现，于2013年获得国家优秀自费留学生奖学金。迄今在Nat. Commun.、J. Am. Chem. Soc.、Angew. Chem. Int. Ed.、ACS Nano、Mater. Horiz.、NPG Asia Mater.、Nano Res.、J. Phys. Chem. Lett.、Nanoscale和Chem. Commun.等期刊发表SCI收录的论文40余篇（一作/通讯21篇），有10篇（一作论文5篇）论文进入ESI TOP1%“高被引论文”；在英国皇家化学会发表专著章节一章。截至2017年9月，论文引用2400 余次，H-index 为24 (Google scholar: https://scholar.google.com/citations?user=Qa7-OwMAAAAJ&hl=zh-CN)。
一、学习工作经历
2017年9月至今，青岛科技大学特聘教授
2014.02‒2017.08，博士后&研究科学家，新加坡生物工程和纳米技术研究所，导师：Jackie Ying教授
2010.01‒2014.01，攻读博士学位，新加坡国立大学，导师：Jianping Xie教授
2006.09‒2009.07，攻读硕士学位，山东理工大学，导师：禚淑萍教授、邢伟教授
2002.09‒2006.07，攻读学士学位，山东理工大学
二、研究方向
1、金属纳米团簇的合成与表征
2、金属纳米团簇在环境、催化、生物医学、能源转化等方面的应用
3、无机纳米多功能材料的制备和表征
三、近年发表论文
1.       Q. Yao,† X. Yuan,† V. Fung, Y. Yu, D. T. Leong, D. Jiang, and J. Xie. Understanding Seed-Mediated Growth of Gold Nanoclusters at Molecular Level. Nat. Commun. 2017, accepted. (†共同一作; JCR一区; IF: 12.12)
2.       N. Goswami, Z. Luo, X. Yuan,* D. T. Leong, and J. Xie*, Engineering gold-based radiosensitizers for cancer radiotherapy. Mater. Horiz., 2017, 4(5), 817-831. (JCR一区; IF: 10.70)
3.       X. Yuan, B. Zhang, Z. Luo, Q. Yao, D. T. Leong, N. Yan, and J. Xie. Balancing the Rate of Cluster Growth and Etching for Gram-Scale Synthesis of Thiolate-Protected Au25 Nanoclusters with Atomic Precision. Angew. Chem. Int. Ed. 2014, 53(18),  4623-4627. (JCR一区; 高被引论文; IF: 11.99; 引用: 105)
4.       X. Yuan, Z. Luo, Q. Zhang, X. Zhang, Y. Zheng, J. Y. Lee, and J. Xie. Synthesis of Highly Fluorescent Metal (Ag, Au, Pt, and Cu) Nanoclusters by Electrostatically Induced Reversible Phase Transfer. ACS Nano 2011, 5(11),  8800-8808. (JCR一区; 高被引论文; IF: 13.94; 引用: 213)
5.       X.  Yuan, M. I. S. Setyawati, A. S. Tan, C. N. Ong, D. T. Leong, and J. Xie. Highly Luminescent Silver Nanoclusters with Tunable Emissions: Cyclic Reduction-Decomposition Synthesis and Antimicrobial Property. NPG Asia Mater. 2013, 5, e39; doi:10.1038/am.2013.3. (JCR一区; 2014-2016年高被引论文; IF: 9.15; 引用: 91)
6.       K. Zheng, X. Yuan,* and J. Xie,* Effect of Ligand Structure on the Size Control of Mono- and Bi-Thiolate-Protected Silver Nanoclusters. Chem. Commun., 2017, 53(70), 9697-9700. (JCR一区; IF: 6.31; 内封面)
7.       X. Yuan, N. Goswami, W. L. Chen, Q. Yao, and J. Xie. Insight into the Effect of Surface Ligands on the Optical Properties of Thiolated Au25 Nanoclusters. Chem.  Commun. 2016, 52(30), 5234-5237. (JCR一区; 高被引论文; 内封面; IF: 6.31; 引用: 16)
8.       X. Yuan, N. Goswami, I. Mathews, Y. Yu, and J. Xie. Enhancing Stability Through Ligand-Shell Engineering: A Case Study with Au25(SR)18 Nanoclusters. Nano Res. 2015,  8(11), 3488-3495. (JCR一区; IF: 7.35; 引用: 13)
9.       K. Zheng,† X. Yuan,† K. Kuah, Z. Luo, Q. Yao, Q. Zhang, and J. Xie. Boiling Water Synthesis of Ultrastable Thiolated Silver Nanoclusters with Aggregation-Induced Emission. Chem. Commun.2015, 51(82), 15165-15168. (†共同一作; JCR一区; IF: 6.31; 引用: 24)
10.    X. Yuan, X. Dou, K. Zheng, and J. Xie. Recent Advances in the Synthesis and Applications of Ultrasmall Bimetallic Nanoclusters. Part. Part. Syst. Charact. 2015, 32(6), 613–629. (邀约综述; IF: 4.47; 引用: 21)
11.    X. Yuan,  M. I. S. Setyawati, D. T. Leong, and J. Xie. Ultrasmall Ag+-Rich Nanoclusters as Highly Efficient Nanoreservoirs for Bacterial Killing. Nano Res. 2014, 7(3), 301-307. (JCR一区; IF: 7.35; 引用: 45)
12.    X. Dou,† X. Yuan,† Y. Yu, Z. Luo, Q. Yao, D. Leong, and J. Xie. Lighting Up Bimetallic Au@Ag Nanoclusters via Aggregation-Induced Emission. Nanoscale 2014, 6(1), 157-161. († 共同一作; JCR一区; 2015-2016年高被引论文; IF:7.36; 引用: 64)
13.    X. Yuan, Q. Yao, Y. Yu, Z. Luo, X. Dou, and J. Xie. Traveling through the Desalting Column Spontaneously Transforms Thiolated Ag Nanoclusters from Nonluminescent to Highly Luminescent. J. Phys. Chem. Lett. 2013, 4(11), 1811–1815. (JCR一区； RSC ChemistryWorld作亮点报道http://www.rsc.org/chemistryworl ... s-purification-xie; IF: 9.35; 引用: 18)
14.    X.  Yuan, Y. Tay, X. Dou, Z. Luo, D. T. Leong, and J. Xie. Glutathione-Protected  Silver Nanoclusters as Cysteine-Selective Fluorometric and Colorimetric  Probe. Anal. Chem. 2013, 85(3), 1913-1919.(JCR一区; 高被引论文; IF: 6.32; 引用: 152)
15.    X. Yuan, Z. Luo, Y. Yu, Q. Yao, and J. Xie. Luminescent Noble Metal Nanoclusters as an Emerging Optical Probe for Sensor Development. Chem. Asian J. 2013, 8(5), 858-871. (高被引论文; 邀约综述; IF: 4.08; 引用: 140)
16.    X. Yuan, Y. Yu, Q. Yao, Q. Zhang, and J. Xie. Fast Synthesis of Thiolated Au25 Nanoclusters via Protection-Deprotection Method.J. Phys. Chem. Lett. 2012, 3(17), 2310-2314. (JCR一区; IF: 9.35; 引用: 43)
17.    X. Yuan, T. J. Yeow, Q.  Zhang, J. Y. Lee, and J. Xie. Highly Luminescent Ag+ Nanoclusters for Hg2+ Ion Detection. Nanoscale 2012, 4(6), 1968-1971. (JCR一区; IF: 7.36; 引用: 85)
18.    X.  Yuan,  W. Xing, S. P. Zhuo, Z. H. Han, G. Q. Wang, et al. Preparation and Application of Mesoporous Fe/Carbon Composites as a Drug Carrier. Micropor. Mesopor. Mat. 2009, 117(3), 678-684. (IF: 3.61; 引用: 46)
19.    X. Yuan,  W. Xing, S. P. Zhuo, W. J. Si, X. L. Gao, et al. Adsorption of Bulky Molecules of  Nonyphenol Ethoxylate on Ordered Mesoporous Carbons. J.Colloid Interf. Sci.2008,322(2), 558-565.(IF:4.23; 引用: 22)
20.    X. Yuan, S. P. Zhuo, W. Xing, H. Y. Cui, X. D. Dai, et al. Aqueous Dye Adsorption on Ordered Mesoporous Carbons. J. Colloid Interf. Sci. 2007, 310(1), 83-89. (IF: 4.23; 引用: 153)
21.    X. Yuan, Y. Y. Liu, S. P. Zhuo, W. Xing, Y. Q. Sun, et al. Synthesis of Ordered Mesoporous Carbon and its Application in Aqueous Macromolecular Adsorption. Acta Chim. Sin. 2007, 65(17), 1814-1820. (IF: 2.13, in Chinese; 引用：7)
22.    Q. Yao, X. Yuan, Y. Yu, Y. Yu, J. Xie, and J. Y. Lee. Introducing Amphiphilicity to Noble Metal Nanoclusters via Phase-Transfer Driven Ion-Pairing Reaction. J. Am. Chem. Soc. 2015, 137(5), 2128-2136. (JCR一区; 高被引论文; IF: 13.85; 引用: 50)
23. Z. Luo, X. Yuan, Y. Yu, Q. Zhang, D. T. Leong, J. Y. Lee, and J. Xie. From Aggregation-Induced Emission of Au(I)-Thiolate Complexes to Ultra-Bright Au(0)@Au(I)-Thiolate Core-Shell Nanoclusters. J. Am. Chem. Soc. 2012, 134(40), 16662-16670. (JCR一区; 高被引论文; Noteworthy Chemistry ACS作亮点报道; IF: 13.85; 引用: 384)
24.    M. I. Setyawati, X. Yuan, J. Xie, and D. T. Leong. The Influence of Lysosomal Stability of Silver Nanomaterials on Their Toxicity to Human Cells.  Biomaterials 2014, 35(25), 6707-6715. (JCR一区; IF: 8.40; 引用: 72)
25.    X. Dou, X. Yuan, Q. Yao, Z. Luo, K. Zheng, and J. Xie. Facile Synthesis of Water-Soluble Au25–xAgx Nanoclusters Protected by Mono- and Bi-Thiolate Ligands. Chem. Commun. 2014, 50(56), 7459-7462. (JCR一区; IF: 6.31; 引用：24)
26.    K. Zheng, X. Yuan, N. Goswami, Q. Zhang, and J. Xie. Recent Advances in the Synthesis, Characterization, and Biomedical Applications of Ultrasmall Thiolated Silver Nanoclusters. RSC  Adv. 2014, 4(105), 60581-60596. (邀约综述; IF: 3.10; 引用: 53)
27.    J. Zhou, X. Yuan, W. Xing, W. J. Si, S. P. Zhuo. Capacitive Performance of Mesoporous Carbons Derived from the Citrates in Ionic Liquid. Carbon 2010, 48(10), 2765-2772. (JCR一区; IF: 6.33; 引用: 42)
28.    J. Zhou, X. Yuan, W. Xing, W. J. Si, S. P. Zhuo. Mesoporous Carbons Derived from Citrates for Use in Electrochemical Capacitors. New Carbon Mater. 2010, 25(5), 370-375. (IF: 1.02; 引用: 13)
29.    W. Xing, X. Yuan, S. P. Zhuo, C. C. Huang. Preparation of Polyaniline-Coated Mesoporous Carbon and its Enhanced Electrochemical Properties. Polym. Advan. Technol. 2009, 20(12), 1179-1182. (IF: 1.29; 引用: 8)
30.    Q. Yao, Y. Yu, X. Yuan, Y. Yu, D. Zhao, J. Xie, and J. Y. Lee. Counterion‐Assisted Shaping of Nanocluster Supracrystals. Angew. Chem. Int. Ed. 2015, 54(1), 184-189. (JCR一区; IF: 11.99; 引用: 24)
31.    Q. Yao, Z. Luo, X.Yuan, Y. Yu, C. Zhang, J. Xie, and J. Y. Lee. Assembly of Nanoions via the Elec trostatic Interactions: Observation of the Ionic-Like Behavior of Charged Noble Metal Nanoclusters. Sci. Rep.2014, 4, 3848. (IF: 4.25; 引用: 17)
32.    Q. Yao, Y. Yu, X. Yuan, Y. Yu, J. Xie, and J. Y. Lee. Two-Phase Synthesis of Small Thiolate-Protected Au15 and Au18  Nanoclusters. Small 2013, 9(16), 2696-2701. (JCR一区; IF: 8.64; 引用: 36)
33.    T. Chen, Q. Yao, X. Yuan, R. R. Nasaruddin, and J. Xie. Heating or Cooling: Temperature Effects on the Synthesis of Atomically Precise Gold Nanoclusters  J. Phys. Chem. C 2017, 121 (20), 10743-10751 (特刊约稿; IF: 4.53)
34.    J. Fang, J. Li, B. Zhang, X. Yuan, H. Asakura, T. Tanaka, K. Teramura, J. Xie, and N. Yan. The Support Effect on the Size and Catalytic Activity of Thiolated Au25 Nanoclusters as Precatalyst. Nanoscale 2015, 7(14), 6325-6333. (JCR一区; 高被引论文; IF:7.36; 引用: 39)
35.    M. I. Setyawati, R. V. Kutty, C. Y. Tay, X. Yuan, J. Xie, and D. T. Leong. Novel Theranostic DNA Nanoscaffolds for the Simultaneous Detection and Killing of Escherichia coli and Staphylococcus aureus. ACS Appl. Mater. Interfaces 2014, 6(24), 21822-21831. (JCR一区; IF: 7.50; 引用: 21)
36.    Y. Yu, Q. Yao, K. Cheng, X. Yuan, Z. Luo, and J. Xie. Solvent Controls the Formation of Au29(SR)20 Nanoclusters in the CO-Reduction Method. Part. Part. Syst. Charact. 2014, 31(6), 652-656. (IF: 4.47; 引用: 10)
37.    Y. Yu, Q. Yao, Z. Luo, X. Yuan, J. Y. Lee, and J. Xie. Precursor Engineering and Controlled Conversion for the Synthesis of Monodisperse Thiolate-Protected Metal Nanoclusters. Nanoscale 2013, 5(11), 4606-4620. (JCR一区; 邀约综述; IF: 7.36; 引用：68)
38. W. Xing, C. C. Huang, S. P. Zhuo, X. Yuan, G. Q. Wang, et al. Hierarchical Porous Carbons with High Performance for Supercapacitor Electrodes. Carbon 2009, 47(7), 1715-1722. (JCR一区; 高被引论文; IF: 6.33; 引用: 252)
39.    W. Xing, S. P. Zhuo, X. L. Gao, and X. Yuan. Adsorption Behavior of NPE on Ordered Mesoporous Carbons. Acta Chim. Sin. 2009, 67(2), 1771-1778. (IF: 2.13, in Chinese; 引用: 1)
40.    W. Xing, S. P. Zhuo, W. Si, and X. Yuan. Preparation of Magnetic Ordered Mesoporous Carbon and Its Drug Adsorption Behavior. Acta Chim. Sin. 2009, 67(8), 761-766. (IF: 2.13, in Chinese; 引用: 6)
41.    X. D. Zhang, Z. Luo, J. Chen, S. Song, X. Yuan, X. Shen, et al. Ultrasmall Glutathione-Protected Gold Nanoclusters as Next Generation Radiotherapy Sensitizers with High Tumor Uptake and High Renal Clearance. Sci. Rep.2015, 5, 8669. (高被引论文; IF: 4.25; 引用: 60)
42.    W. Xing, S. P. Zhuo, H. Cui, H. Zhou, W. Si, X. Yuan, X. Gao, and Z. Yan. Morphological Control in Synthesis of Cobalt Basic Carbonate Nanorods Assembly. Mater. Lett. 2008, 62(8), 1396-1399. (IF: 2.57; 引用: 5)
四、专著章节
1.       X. Yuan, Q. Yao, Y. Yu, Z. Luo, and J. Xie. Novel Synthetic Strategies for Thiolate-Protected Au and Ag Nanoclusters: Towards Atomic Precision and Strong Luminescence. In RSC Book Smart Materials "Functional Nanometer-Sized Clusters of Transition Metals: Synthesis, Properties and Applications" 2014, ISBN: 978-1-84973-824-8.

baozhang · 发表于 2021-11-17 15:16:13

贵金属纳米团簇作为一类新型的功能纳米材料，在催化、能源转化、传感、生物医学等领域备受关注。从原子级别精确的团簇的设计合成、理化性质研究，到相关领域的应用，无不蕴含着广大研究者的智慧。当前，贵金属纳米团簇的发展机遇与挑战并存，适时地总结过往的研究经验和最新的研究进展能进一步促进团簇领域的发展。基于此，材料学院泰山青年学者袁勋教授领衔的贵金属纳米团簇课题组聚焦于金属纳米团簇的合成、性质研究、光催化及传感应用，今年以来连续受邀在化学权威综述期刊Coordination Chemistry Reviews（IF: 22.315）撰写综述论文2篇，同时与新加坡国立大学合作分别在材料学权威期刊Nano Energy（IF: 17.881）和化学权威期刊Chemical Science（IF: 9.825）撰写综述论文各1篇，以实际行动助力学校高水平大学建设。

      今年1月，袁勋教授与新加坡国立大学谢建平教授、姚桥峰研究员合作在化学权威期刊《Chemical Science》上发表了题为“Molecular reactivity of thiolate-protected noble metal nanoclusters: synthesis, self-assembly, and applications”的综述论文，就金属纳米团簇的分子反应活性对团簇合成、自组装及应用进行了详尽评述，为深入理解金属纳米团簇的类分子理化性质提供了有益信息。袁勋教授与新加坡国立大学谢建平教授为论文的共同通讯作者，新加坡国立大学姚桥峰研究员为论文的第一作者。
   4月，团队在《Coordination Chemistry Reviews》上发表的题为“The beauty of binary phases: a facile strategy for synthesis, processing, functionalization, and application of ultrasmall metal nanoclusters”的综述，文章系统的总结了过去10年里，水-油两相策略在团簇合成、处理、功能化及应用等方面的巧妙运用，并就这一策略在未来的研究工作中的应用进行了展望。袁勋教授为该论文唯一通讯作者，博士生王子平为第一作者，我校为第一通讯单位。
7月，团队与新加坡国立大学合作在材料学权威期刊《Nano Energy》上发表了题为“Shining photocatalysis by gold-based nanomaterials”的综述论文，就金纳米颗粒和金纳米团簇材料在光催化应用中的飞速发展做了适时的评述与总结。该工作例证了金纳米材料的引入可以很好的解决传统半导体光催化的关键限制，梳理了纳米金修饰光催化剂的制备方法；讨论了金纳米材料在光催化过程中的提高光催化性能的机理，并对纳米金修饰光催化剂在太阳能转换、环境修复和有机合成等方面的应用进展进行了综述。该工作阐明了高性能金属掺杂的半导体光催化剂的设计原则，可有效促进该领域的进一步发展。我校材料学院袁勋教授与新加坡国立大学谢建平教授、姚桥峰研究员为该论文共同通讯作者，材料学院朱海光副教授为第一作者，我校为第一通讯单位。
      日前，团队再次受邀在化学权威期刊《Coordination Chemistry Reviews》上发表了题为“Engineering luminescent metal nanoclusters for sensing applications”的综述论文，对金属纳米团簇基荧光传感器的研究进展进行了评述。该工作在金属纳米团簇设计与荧光传感器构筑之间架起了桥梁，全面总结了金属纳米团簇影响荧光传感器性能的理化性质，归纳了合成强荧光纳米团簇的主要策略，并就团簇基传感器的构造及工作机理进行了全新解析。袁勋教授为该论文唯一通讯作者，硕士生钱树钰为第一作者，我校为第一通讯单位。
      该系列论文的发表离不开团队成员多年来在团簇领域的辛勤耕耘，更离不开院校两级单位对金属纳米团簇创新团队的支持。另外，该系列论文也获得了国家自然科学基金面上项目、泰山学者青年专家专项基金、山东省优秀青年基金等项目资助。
   《Coordination Chemistry Reviews》即《配位化学评论》，由国际著名学术出版集团Elsevier发行，是目前化学学科最具权威性的综述性学术期刊之一，2021年最新影响因子为22.315。重点刊登配位化学、过渡金属化学、主族元素化学、金属有机化学、材料化学、生物无机化学等领域的综述论文。

论文链接：
(1)Yao Qiaofeng, Wu Zhennan, Liu Zhihe, Lin Yingzheng, Yuan Xun*, Xie Jianping*. Molecular reactivity of thiolate-protected noble metal nanoclusters: synthesis, self-assembly, and applications.Chem. Sci.2021, 12, 99. (链接:https://pubs.rsc.org/en/content/articlelanding/2021/SC/D0SC04620E)
(2)Wang Ziping, Pan Xinxin, Qian Shuyu, Yang Ge, Du Fanglin, Yuan Xun*. The beauty of binary phases: A facile strategy for synthesis, processing, functionalization, and application of ultrasmall metal nanoclusters.Coordin. Chem. Rev.2021, 438, 213900. (链接:https://www.sciencedirect.com/sc ... i/S001085452100134X)
(3)Zhu Haiguang, Yuan Xun*, Yao Qiaofeng*, Xie Jianping*. Shining photocatalysis by gold-based nanomaterials.Nano Energy2021, 88, 106306. (链接:https://www.sciencedirect.com/sc ... i/S2211285521005619)
(4)Qian Shuyu, Wang Ziping, Zuo Zhongxiang, Wang Xiaomeng, Wang Qing, Yuan Xun*. Engineering luminescent metal nanoclusters for sensing applications.Coordin. Chem. Rev.2022, 214268. (链接:https://www.sciencedirect.com/sc ... i/S0010854521005427)

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[专家学者] 青岛科技大学材料学院袁勋

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