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姓名：王彦广
单位：化学系
职称：教授
兰州大学化学系学士（1981-1985)、硕士（1985-1988) 和博士（1990-1993)，浙江大学博士后（1994-1995)及香港中文大学博士后（1997-1998)。1988-1993年任天津大学化学系教师，1993年晋升为副教授。1995年10月至今任浙江大学化学系教师，1998年晋升为教授。曾任浙江大学化学系主任（1999-2005; 2010-2017)，浙江大学理学院副院长（2005-2009），浙江省化学会副理事长（2002-2010)。现兼任浙江省化学会理事长（2010-迄今)，中国化学会理事，《高等学校化学学报》、《Chemical Research in Chinese Universities》、《应用化学》和《大学化学》期刊编委，国家自然科学基金委员会专家评审组成员，教育部高等学校化学类专业教学指导委员会委员。主要从事有机合成化学以及药物化学研究, 在JACS、CC、JOC、OL等国际著名期刊上发表论文160余篇，编著教材、专著5部。获浙江省高等学校教学名师奖（2011）、宝钢优秀教师奖(2009)、教育部高校青年教师奖（2003)和中国化学会青年化学奖（1999）等奖励。
工作研究领域
（1）有机合成新反应和新方法研究 （2）生物活性天然产物及其类似物的合成 （3）药物化学
联系方式
电话：0571-87951512; 13588861496
电子信箱：orgwyg@zju.edu.cn
专利
1 林旭锋，崔孙良，王彦广，3-位含有芳基取代基的1,2,4-噁二唑啉及其固相合成法，中国发明专利：ZL 03116520.6, 授权公告日：2005-05-18; 申请日：2003-04-17; 证书号：209426.
2 林旭锋，张健，王彦广，5位含有酯基的1,3-芳基取代的吡唑啉液相合成法，中国发明专利：ZL 03129682.3, 授权公告日：2005-09-21; 申请日：2003-06-30; 证书号：228452.
3 林旭锋，丁寒锋，王彦广，5位含有酯基的1,3-芳基取代的吡唑及其液相合成法，中国发明专利：ZL 03129683.1, 授权公告日：2005-11-23; 申请日：2003-06-30; 证书号：236886.
4 崔孙良，林旭锋，王彦广，2,6-二氰基苯胺衍生物的微波合成方法，中国发明专利：ZL 200410073484.9, 授权公告日：2006-07-26; 申请日：2004-12-21; 证书号：275210.
5、崔孙良，林旭锋，王彦广，2,6-二氰基苯胺衍生物的制备方法，中国发明专利：ZL 200410084349.4, 授权公告日：2006-08-23; 申请日：2004-11-16; 证书号：279714.
6 雷鸣，王彦广，1,3-二取代咪唑-2-硫酮的微波合成方法，中国发明专利：ZL 200510050465.9, 授权公告日：2007-01-10; 申请日：2005-06-27; 证书号：
7 雷鸣，王彦广，微波辐射合成1,3-二取代咪唑-2-硫酮，中国发明专利：ZL 200510049201.1, 授权公告日：2007-02-14; 申请日：2005-01-24; 证书号：
8 林旭锋，崔孙良，王彦广，一种六氢呋喃[3,2-c]喹啉衍生物的制备方法，中国发明专利ZL 200610050521.3, 授权公告日：2008-03-26; 申请日：2006-04-26; 证书号：385336.
9 林旭锋，崔孙良，王彦广，一种二吲哚甲烷衍生物的制备方法，中国发明专利ZL 200610050520.9, 授权公告日：2008-03-26; 申请日：2006-04-26; 证书号：385331.
10 林旭锋，崔孙良，王彦广，一种3位取代吲哚衍生物的制备方法，中国发明专利ZL 200610050393.2, 授权公告日：2008-06-04；申请日：2006-04-18; 证书号：400599.
11 陈正波，洪灯，陆伟，王彦广，林旭锋，2位含有酯基的3-芳基取代吲哚的制备方法，中国发明专利ZL 200910096596.9，授权公告日：2011-06-15；申请日：2009-03-10; 证书号：797065.
12 洪灯，朱元勋，林旭峰，雷鸣，王彦广，一种四氢三嗪衍生物的制备方法，中国发明专利ZL 200910100675.2，授权公告日：2011-08-24；申请日：2009-07-16; 证书号：829135.
13 韩超，沈阳，徐方曦，吕萍，王彦广，一种促代谢型谷氨酸受体增强剂类似物及其制备方法，中国发明专利ZL201210063585.2，授权公告日：2014-04-16；申请日：2012-03-12; 证书号：1383218.
14 吕萍，王彦广，温俏冬，金继松，一种由芳基卤化物制备芳基腈的方法，中国发明专利ZL201210383415.2，授权公告日：2014-08-06；申请日：2012-10-11; 证书号：1455802.
15 李继超，李熙晖，吕萍，王彦广，一种检测[H+]的荧光化学传感器及其制备和使用方法，中国发明专利ZL 201110220376.X，授权公告日：2013-09-04；申请日：2011-08-03; 证书号：1267616.
16 胡彬彬，李继超，胡公方，吕萍，王彦广，一种基于吡咯甲川衍生物的pH比色检测分析方法，中国发明专利ZL 201210008864.9，授权公告日：2013-09-04；申请日：2012-01-12; 证书号：1267259.
17 钟建华，沈莉萍，王彦广, 秋水仙碱衍生物，中国发明专利ZL201210318831.4，授权公告日：2015-02-25; 申请日：2012-09-03；证书号：1594952.
论文
1. Guorong Sheng, Shicong Ma, Songlin Bai, Jianming Mao, Ping Lu * and Yanguang Wang, A copper-catalyzed reaction of 3-diazoindolin-2-imines with 2-(phenylamino)ethanols: convenient access to spiro[indoline-3,20’-oxazolidin]-2-imines, Chem. Commun. 2018, 54, 1529-1532.
2. Fanghui Ma, Jing Qian, Ping Lu,* and Yanguang Wang*, Convenient Synthesis of 2-Amino-3-(arylthio)indoles via Rh-Catalyzed Reaction of 3-Diazoindol-2-imines with Thioesters, Organic & Biomolecular Chemistry 2018, 16, 439-443.
3. Jie Qi, Zaibin Wang, Bo Lang, Ping Lu,* and Yanguang Wang*, TfOH-Catalyzed Reaction between 3-Diazoindolin-2-imines and Electron-Rich Arenes: Access to 3-Aryl-2-aminoindoles, J. Org. Chem. 2017, 82(23), 12640-12646.
4. Lang Sun, Peng Liu, Jing Wang, Ping Lu,* and Yanguang Wang*, Preparation of Spiro[indene-1,1’-isoindolin]-3'-ones via Sulfuric Acid-Promoted Cascade Cyclization, J. Org. Chem. 2017, 82(16), 8407-8418.
5. Kai Huang, Guorong Sheng, Ping Lu,* and Yanguang Wang*, BF3-Promoted Divergent Reactions between Tryptophols and Propargylic Alcohols, Org. Lett. 2017, 19(15), 4114-4117.
6. Kai Huang, Guorong Sheng, Ping Lu,* and Yanguang Wang*, From 1-Sulfonyl-4-aryl-1,2,3-triazoles to 1-Allenyl-5-aryl-1,2,3-Triazoles, J. Org. Chem. 2017, 82(10), 5294-5300.
7. Zhixing Peng, Kai Huang, Yuhan Tao, Xihui Li, Lianpeng Zhang, Ping Lu,* and Yanguang Wang*, Turning on the solid emission from non-emissive 2-aryl-3-cyanobenzofurans by tethering tetraphenylethene for green electroluminescence, Mater. Chem. Front. 2017, 1(9), 1858-1865.
8. Xihui Li, Jiaming Li, Yuhan Tao, Zhixing Peng, Ping Lu,* and Yanguang Wang*, Oxazole-based high resolution ratiometric fluorescent probes forhydrogen peroxide detection, Sensors and Actuators B 2017, 247, 609–616.
9. Anni Ren, Bo Lang, Jialun Lin, Ping Lu,* and Yanguang Wang*, 4-Diazoisochroman- 3-imines: A Class of Metal Carbene Precursors for the Synthesis of Isochromene Derivatives, J. Org. Chem. 2017, 82(20), 10953−10959.
10. Bo Lang, Huangtianzhi Zhu, Chen Wang, Ping Lu,* Yanguang Wang*, Rhodium-Catalyzed Cycloadditions between 3-Diazoindolin-2-imines and 1,3-Dienes, Org. Lett. 2017, 19, 1630-1633.
11. Anni Ren, Ping Lu* and Yanguang Wang*, Convenient preparation of 4-diazoisochroman-3-imines and 3-subsituted 3,5-dihydroisochromeno- [3,4-d][1,2,3]triazoles, Chem. Commun. 2017, 53, 3769-3772.
12. Xiaorong Zhou, Zhiyin Zhang, Hongyang Zhao, Ping Lu,* and Yanguang Wang*, Rh-Catalyzed Annulations of N-Methoxybenzamides and Ketenimines: Sterically and Electronically Controlled Synthesis of Isoquinolinones and Isoindolinones, J. Org. Chem.2017, 82, 3787-3797.
13. Hualong Ding, Songlin Bai, Ping Lu,* and Yanguang Wang*, Preparation of 2-Amino-3-arylindoles via Pd-Catalyzed Coupling between 3-Diazoindolin-2-imines and Arylboronic Acids as well as Their Extension to 3-Aryl-3-fluoroindolin-2-imines, Org. Lett. 2017, 19, 4604-4607.
14. Hualong Ding,Zaibin Wang, Songlin Bai, Ping Lu,* and Yanguang Wang*, Rh-Catalyzed Conversion of 3-Diazoindolin-2-imines to 5H-Pyrazino[2,3-b]indoles with Photoluminescent Properties, Org. Lett. 2017, 19, 6514–6517.
15. Xiaorong Zhou, Zhixing Peng, Hongyang Zhao, Zhiyin Zhang, Ping Lu*, Yanguang Wang*, Rh-Catalyzed annulations of N-methoxybenzamides with ketenimines: synthesis of 3-aminoisoindolinones and 3-diarylmethyleneisoindolinones with strong aggregation induced emission properties, Chem. Commun. 2016, 52, 10676-10679
16. Xiaorong Zhou, Zili Fan, Zhiyin Zhang, Ping Lu,* Yanguang Wang*， Construction of Pyrrolo[1,2-a]indoles via Cobalt(III)-Catalyzed Enaminylation of 1-(Pyrimidin-2-yl)-1H-indoles with Ketenimines and Subsequent Base-Promoted Cyclization，Org. Lett. 2016, 18, 4706-4709.
17. Hongyang Zhao, Yanpeng Xing, Ping Lu,* Yanguang Wang*, Synthesis of 2,3-Disubstituted Quinolines via Ketenimine or Carbodiimide Intermediates, Chem. Eur. J.2016, 22, 15144-15150.
18. Jing Qian, Guorong Sheng, Kai Huang, Shaojie Liu, Ping Lu*, Yanguang Wang*, a-Amidino Rhodium Carbenes: Key Intermediates for the Preparation of (E)-2-Aminomethylene-3-oxoindoles and Pyranoindoles, Org. Lett. 2016, 18 (15), 3682–3685.
19. Zhenmin Li, Xiaorong Zhou, Ping Lu*, Yanguang Wang*, Preparation of 3-Aryl-2-aminoindoles via Rhodium-Catalyzed Coupling Reaction between 2-Arylpyridines and 3-Diazoindolin-2-imines, J. Org. Chem. 2016, 81, 9433-9437.
20. Lianpeng Zhang, Zhixing Peng, Qiaodong Wen, Xihui Li, Ping Lu*, Yanguang Wang*, Copper-Catalyzed Preparation of 2-Aryl-3-cyanobenzofurans with Bright Blue Photoluminescence, Org. Lett. 2016, 18 (4), 728–731.
21. Lianpeng Zhang, Xin Gu, Ping Lu *, Yanguang Wang*, Synthesis of a-aminonitriles via a FeSO4-mediated oxidative cyanation of tertiary amines with benzoyl cyanide and molecular oxygen or TBHP, Tetrahedron 2016, 72, 2359-2363.
22. Hualong Ding, Zhixing Peng, Jinjin Wang, Ping Lu*, Yanguang Wang*, Preparation of 3-azoindoles and 3-hydrazonoindolin-2-imines as well as their applications as NNO pincer ligands for boron, Org. Biomol. Chem. 2016, 14, 7114–7118.
23. Qiaodong Wen, Ping Lu*, Yanguang Wang*, Copper-mediated three-component synthesis of 3-cyanoimidazo[1,2-a]pyridines, Chem. Commun. 2015, 51, 15378-15381.
24. Guorong Sheng, Kai Huang, Shicong Ma, Jing Qian, Ping Lu*, Yanguang Wang*, Preparation of 3-aryl-2-aminoindoles, 3-allyl-3-amino-2-iminoindolines, and tetrahydro-[1,4]diazepino[2,3-b]indoles from 3-diazoindolin-2-imines, Chem. Commun. 2015, 51, 11056-11059.
25. Lianpeng Zhang, Ping Lu*, Yanguang Wang*, Cu(NO3)2-3H2O-mediated cyanation of aryl iodides and bromides using DMF as a single surrogate of cyanide, Chem. Commun. 2015, 51, 2840-2843.
26. Chen Wang, Haojie Zhang, Bo Lang, Anni Ren, Ping Lu*, Yanguang Wang*, Rh-Catalyzed Reactions of 3-Diazoindolin-2-imines: Synthesis of Pyridoindoles and Tetrahydrofuropyrroloindoles, Org. Lett. 2015, 17(18), 4412-4415.
27. Jinjin Wang, Jiyong Liu, Hualong Ding, Jing Wang, Ping Lu*, Yanguang Wang*, Construction of Multifunctional 3-Amino-2-carbamimidoylacrylamides and Their Crystalline Channel-Type Inclusion Complexes, J. Org. Chem. 2015, 80(11), 5842-5850.
28. Xiaorong Zhou, Zheng Jiang, Lexing Xue, Ping Lu*, Yanguang Wang*, Preparation of 1,2,5-Trisubstituted 1H-Imidazoles from Ketenimines and Propargylic Amines by Silver-Catalyzed or Iodine-Promoted Electrophilic Cyclization Reaction of Alkynes, Eur. J. Org. Chem. 2015, 5789–5797.
29. Lianpeng Zhang, Ping Lu*, Yanguang Wang*, Copper-mediated cyanation of indoles and, electron-rich arenes using DMF as a single surrogate, Org. Biomol. Chem. 2015, 13(30), 8322–8329.
30. Jinjin Wang, Ping Lu*, Yanguang Wang*, Copper-catalyzed multi-component synthesis of acrylamidines and benzoimidazoles, Org. Chem. Front., 2015, 2, 1346–1351.
31. Du Z, Xing YG, Lu P*, Wang YG*, Copper-Catalyzed Cascade Double C3-Indolations of 3-Diazoindolin-2-imines with Indoles: Convenient Access to 3,3-Diaryl-2-iminoindoles, Org. Lett. 2015,17(5),1192-1195.
32. Sun L, Zhu YX, Wang J, Lu P,* Wang YG*, Lewis Acid Catalyzed Cascade Reaction of 3-(2-Benzenesulfonamide)propargylic Alcohols to Spiro[indenebenzosultam]s, Org. Lett. 2015,17, 242-245.
33. Sheng GR, Huang K, Chi ZH, Ding HL, Yanpeng Xing, Lu P,* Wang YG*, Preparation of -Diazoindolin-2-imines via Cascade Reaction between Indoles and Sulfonylazides and Their Extensions to 2,3-Diaminoindoles and Imidazo[4,5-b]indoles, Org. Lett. 2014, 16(19), 5096-5099.
34. Xing YP, Cheng, BY, Wang J, Lu P*, Wang YG*, Copper-Catalyzed Three-Component Synthesis of 3-Aminopyrazoles and 4-Iminopyrimidines via β-Alkynyl-N-sulfonyl Ketenimine Intermediates, Org. Lett. 2014, 16 (18), 4814–4817.
35. Xing YP, Sheng GR, Wang J, Lu P*, Wang YG*, Preparation of Triazoloindoles via Tandem Copper Catalysis and Their Utilities as α-Imino Rhodium Carbene Precursors, Org. Lett. 2014, 16 (4), 1244–1247.
36. Zhu YX, Sun L, Lu P*, Wang YG*, Recent Advances on the Lewis Acid-Catalyzed Cascade Rearrangements of Propargylic Alcohols and Their Derivatives, ACS Catal. 2014, 4, 1911-1925. (Review)
37. Wang JJ, Wang J, Lu P*, Wang YG*, Copper-Catalyzed Cascade Preparation of Dihydropyrimidin-4-ones from N-(Prop-2-yn-1-yl)amides and Azides. J. Org. Chem. 2013, 78(17), 8816-8820.
38. Xing YP, Hu BB, Yao QJ, Lu P*, Wang YG*, Tandem Synthesis of Benzocarbazoles and Their Photoluminescent Properties. Chem. Eur. J. 2013, 19(38), 12788-12793.
39. Sun L, Zhu YX, Lu P*, Wang YG*, Cu-Catalyzed 1,2-Dihydroisoquinolines Synthesis from o-Ethynyl Benzacetals and Sulfonyl Azides, Org. Lett. 2013, 15(22), 5894-5897.
40. Zhang LP, Wen QD, Jin JS, Wang C, Lu P*, Wang YG*, Cyanation of indoles with benzyl cyanide as the cyanide anion surrogate. Tetrahedron 2013, 69(21), 4236-4240.
41. Yin GW, Zhu YX, Wang NN, Lu P*, Wang YG*, Lewis acid-promoted cascade reaction of primary amine, 2-butynedioate, and propargylic alcohol: a convenient approach to 1,2-dihydropyridines and 1H-pyrrolo 3,4-b pyridine-5,7(2H,6H)-diones. Tetrahedron 2013, 69(39), 8353-8359.
42. Xing YP, Zhao HW, Shang QY, Wang J, Lu P*, Wang YG*, Parallel Copper Catalysis: Diastereoselective Synthesis of Polyfunctionalized Azetidin-2-imines. Org. Lett. 2013, 15(11), 2668-2671.
43. Wen QD, Jin JS, Mei Y, Lu P*, Wang YG*, Copper-Mediated Cyanation of Aryl Halides by Activation of Benzyl Cyanide as the Cyanide Source. Eur. J. Org. Chem. 2013, 2013(19), 4032-4036.
44. Wang NN, Cai SY, Zhou C, Lu P*, Wang YG*, One-pot synthesis of 2-aryl-3-alkoxycarbonyl chromones through a cascade Lewis acid-catalyzed aldehyde olefination/oxa-Michael addition/oxidation. Tetrahedron 2013, 69(2), 647-652.
45. Wang C, Zhang LP, Ren AN, Lu P*, Wang YG*, Cu-Catalyzed Synthesis of Tryptanthrin Derivatives from Substituted Indoles. Org. Lett. 2013, 15(12), 2982-2985.
46. Luo Y, Wen QD, Wu Z, Jin JS, Lu P*, Wang YG*, Copper-mediated cyanation of aryl boronic acids using benzyl cyanide. Tetrahedron 2013, 69(39), 8400-8404.
47. Li JC, Hu GF, Wang NN, Hu T, Wen QD, Lu P*, Wang YG*, Oligo(3,6-phenanthrene ethynylenes): Synthesis, Characterization, and Photoluminescence. J. Org. Chem. 2013, 78(7), 3001-3008.
48. Hu BB, Lu P*, Wang YG*, Fluorescent chemosensors based on 9-cycloheptatrienylidene fluorenes (9-CHFs). New J. Chem. 2013, 37(6), 1645-1653.
49. Hu BB, Chen XP, Wang YF, Lu P*, Wang YG*, Structure-Property Investigations of Substituted Triarylamines and Their Applications as Fluorescent pH Sensors. Chem. Asian J. 2013, 8(6), 1144-1151.
50. Han C, Shen Y, Lu P*, Wang YG*, Palladium-Catalyzed Cyclocarbonylation of 2-Halobenzaldehyde and Hydrazines: A Facile Synthesis of 2-Aminoisoindolin-1-ones. Chin. J. Chem . 2013, 31(2), 182-186.
51. Zhu YX, Yin GW, Sun L, Lu P*, Wang YG*, Tandem reaction of propargyl alcohols and N-tosyl hydroxylamine: switchable synthesis of 2,5-dihydroisoxazoles and 4-halo-2,5-dihydroisoxazoles. Tetrahedron 2012, 68(49), 10194-10200.
52. Zhou C, Chen XP, Lu P*, Wang YG*, Synthesis of 2,3-diiodoindenes and their applications in construction of 13H-indeno 1,2-l phenanthrenes. Tetrahedron 2012, 68(13), 2844-2850.
53. Zhang L, Zhu YX, Yin GW, Lu P*, Wang YG*, 3-Alkenylation or 3-Alkylation of Indole with Propargylic Alcohols: Construction of 3,4-Dihydrocyclopenta b indole and 1,4-Dihydrocyclopenta b indole in the Presence of Different Catalysts. J. Org. Chem. 2012, 77(21), 9510-9520.
54. Xu FX, Huang D, Lin XF*, Wang YG*, Highly enantioselective Biginelli reaction catalyzed by SPINOL-phosphoric acids. Org. Biomol. Chem. 2012, 10(22), 4467-4470.
55. Wen QD, Jin JS, Hu BB, Lu P*, Wang YG*, Palladium-catalyzed cyanide metathesis: utilization of benzyl cyanide as an operator-benign reagent for aryl halide cyanations. Rsc Advances 2012, 2(15), 6167-6169.
56. Shen Y, Han C, Cai SY, Lu P*, Wang YG*, One-pot synthesis of 4(3H)-quinazolinones from azides, alkynes, anilines, and carbon monoxide. Tetrahedron Lett. 2012, 53(42), 5671-5673.
57. Lu P, Wang YG*, The thriving chemistry of ketenimines. Chem. Soc. Rev. 2012, 41(17), 5687-5705. (Review)
58. Li JC, Hu BB, Hu GF, Li X, Lu P*, Wang YG*, An efficient synthesis of heptaaryldipyrromethenes from tetraarylcyclopentadienones and ammonium acetate and their extension to the corresponding BODIPYs. Org. Biomol. Chem. 2012, 10(44), 8848-8859.
59. Jin JS, Wen QD, Lu P*, Wang YG*, Copper-catalyzed cyanation of arenes using benzyl nitrile as a cyanide anion surrogate. Chem. Commun. 2012, 48(79), 9933-9935.
60. Jin JS, Luo Y, Zhou C, Chen XP, Wen QD, Lu P*, Wang YG*, Synthesis of Indeno 1,2-c furans via a Pd-Catalyzed Bicyclization of 2-Alkynyliodobenzene and Propargylic Alcohol. J. Org. Chem. 2012, 77(24), 11368-11371.
61. Jiang Z, Lu P*, Wang YG*, Three-Component Reaction of Propargyl Amines, Sulfonyl Azides, and Alkynes: One-Pot Synthesis of Tetrasubstituted Imidazoles. Org. Lett. 2012, 14(24), 6266-6269.
62. Huang D, Xu FX, Lin XF*, Wang YG*, Highly Enantioselective Pictet-Spengler Reaction Catalyzed by SPINOL-Phosphoric Acids. Chem. Eur. J. 2012, 18(11), 3148-3152.
63. Hu BB, Su Q, Lu P*, Wang YG*, BODIPY modified 9-cycloheptatrienylidene fluorene derivatives: Fluorescent "turn-on" for detecting Cu2+ with acidity independence. Sens. Actuators B, 2012, 168, 310-317.
64. Chen XP, Li XH, Wang NN, Jin JS, Lu P*, Wang YG*, Palladium-Catalyzed Reaction of Arylamine and Diarylacetylene: Solvent-Controlled Construction of 2,3-Diarylindoles and Pentaarylpyrroles. Eur. J. Org. Chem. 2012, 2012(23), 4380-4386.
65. Chen XP, Jin JS, Wang NN, Lu P*, Wang YG*, Palladium-Catalyzed Selective Synthesis of Naphthalenes and Indenones and Their Luminescent Properties. Eur. J. Org. Chem. 2012, 2012(4), 824-830.
66. Chen XP, Lu P*, Wang YG*, Four Iodine-Mediated Electrophilic Cyclizations of Rigid Parallel Triple Bonds Mapped from 1,8-Dialkynylnaphthalenes, Chem. Eur. J. 2011, 17, 8105-8114.
67. Chen XP, Jin JS, Wang YG,* and Lu P* Palladium-Catalyzed Synthesis of 7,9-Diaryl-8H-acenaphtho [1,2-c]pyrroles and Their Application in Explosives Detection，Chem. Eur. J. 2011, 17, 9920-9923.
68. Wang J, Wang JJ, Zhu YX, Lu P*, Wang YG*, Copper-Cascade Catalysis: Synthesis of 3-Functionalized Indoles, Chem. Commun. 2011, 47, 3275-3277.
69. Chen XP, Wang HB, Jin XH, Feng JW, Wang YG*, Lu* P, Palladium catalyzed bicyclization of 1,8-diiodonaphthalene and tertiary propargylic alcohols to phenalenones and their applications as fluorescent chemosensor for fluoride ions, Chem. Comm. 2011, 47 (9), 2628-2630.
70. Lin XF,* Mao ZJ, Dai XX, Lu P, Wang YG*, A straightforward one-pot multicomponent synthesis of polysubstituted Pyrrolesw, Chem. Commun. 2011, 47, 6620–6622.
71. Zhu YX, Wen S, Yin GW, Hong D, Lu P*, Wang YG*, Tandem Reaction of Propargyl Alcohol and N-Sulfonylhydrazone: Synthesis of Dihydropyrazole and Its Utility in the Preparation of 3,3-Diarylacrylonitrile, Org. Lett. 2011, 13(14), 3553-3555.
72. Yin GW, Zhu YX, Zhang L, Lu P*, Wang YG*, Preparation of Allenephosphoramide and Its Utility in the Preparation of 4,9-Dihydro-2H-benzo[f ]isoindoles, Org. Lett. 2011, 13(5), 940–943.
73. Hong D, Zhu YX, Li Y, Lin XF, Lu, P* and Wang YG* Three-Component Synthesis of Polysubstituted Pyrroles from r-Diazoketones, Nitroalkenes, and Amines, Org. Lett. 2011, 13(17), 4668-4671.
74. Zhu YX, Yin GW, Hong D, Lu P*, Wang YG*, Tandem Reaction of Propargylic Alcohol, Sulfonamide, and N-Iodosuccinimide: Synthesis of N-(2-Iodoinden-1-yl)- Arenesulfonamide, Org. Lett. 2011, 13 (5), 1024–1027.
75. Yin GW, Zhu YX, Lu P,* and Wang YG* Lewis Acid-Promoted Three-Component Reactions of Propargylic Alcohols with 2-Butynedioates and Secondary Amines, J. Org. Chem. 2011, 76, 8922-8929.
76. Jiang Z., Wang J., Lu, P*, Wang YG*, Diasteroselective synthesis of oxazolidines and imidazolidines via the Lewis acid catalyzed CeC cleavage of aziridines, Tetrahedron 2011, 67(49), 9609-9617.
77. Shen Y, Cai SY, Chi He, Lin XF*, Lu P, Wang YG*, Three-component reaction for the C2-functionalization of 1-substituted imidazoles with acetylenic ketones and isocyanates, Tetrahedron 2011, 67 (43), 8338-8342.
78. Li Y, Hong D, Zhu YX, Lu P*, Wang YG*, One-pot synthesis of 5-sulfonamidopyrazole from terminal alkynes, sulfonyl azides and hydrozines, Tetrahedron 2011, 67(42), 8086-8090.
79. Jin HW, Zhou ZW, Wu Z, Shen Y, Wang YG*, One-pot synthesis of substituted indolines via a copper-catalyzed sequential multicomponent/CeN coupling reaction, Tetrahedron 2011, 67(6), 1178-1182.
80. Hong D, Zhu YX, Lin XF*, Wang YG*, Facile synthesis of 1,2,4-triazolines via PPh3-triggered reaction of azodicarboxylate with 2-azidoacrylates, Tetrahedron 2011, 67(3), 650-654.
81. Li Y, Hong D, Lu P*, Wang YG*, Synthesis of pyrazoles from 2-azidoacrylates and hydrazonyl chlorides, Tetrahedron Lett. 2011, 52(32), 4161-4163.
82. Cai SY, Shen Y, Lu P*, Wang YG*, Condition-Controlled Selective Synthesis of Coumarins and Flavones from 3-(2-Hydroxyphenyl)propiolates and Iodine, Tetrahedron Lett. 2011, 52(32), 4164-4167.
83. Feng JW, Chen XP, Han QC, Wang HB, Lu P*, Wang YG*, Naphthalene-based fluorophores: Synthesis characterization, and photophysical properties, J. Luminescence 2011, 131, 2775–2783.
84. Song WZ, Lei M, Shen Y, Cai SY, Lu W, Lu P*, Wang YG*, Copper-Catalyzed Four-Component Reaction of Baylis–Hillman Adducts with Alkynes, Sulfonyl Azides and Alcohols, Adv. Synth. Catal. 2010, 352, 2432-2436.
85. Han QC, Su QA, Tang L, Feng JW, Lu P*, Wang YG*, Electron Transfer and Aggregate Formation Coinduced Emission Enhancement of 9-Cycloheptatrienylidene Fluorenes in the Presence of Cupric Chloride, J. Phys. Chem. C 2010, 114(43), 18702-18711.
86. Hong D, Chen ZB, Lin XF*, Wang YG*, Synthesis of Substituted Indoles from 2-Azidoacrylates and ortho-Silyl Aryltriflates, Org. Lett. 2010, 12(20), 4608-4611.
87. Xu FX, Huang D, Han C, Shen W, Lin XF*, Wang YG*, SPINOL-Derived Phosphoric Acids: Synthesis and Application in Enantioselective Friedel-Crafts Reaction of Indoles with Imines, J. Org. Chem. 2010, 75(24), 8677-8680.
88. Jin HW, Xu XL, Gao JR, Zhong JH, Wang YG*, Copper-Catalyzed One-Pot Synthesis of Substituted Benzimidazoles, Adv. Synth. Catal. 2010, 352(2-3), 347-350.
89. Shen Y, Cui SL, Wang J, Chen XP, Lu P*, Wang YG*, Copper-Catalyzed Three-Component Synthesis of 2-Iminodihydrocoumarins and 2-Iminocoumarins, Adv. Synth. Catal. 2010, 352, 1139-1144.
90. Song WZ, Lu W, Wang J, Lu P*, Wang YG*, A Facile Route to γ-Nitro Imidates via Four-Component Reaction of Alkynes with Sulfonyl Azides, Alcohols, and Nitroolefins, J. Org. Chem. 2010, 75, 3481–3483.
91. Su YH, Jiang Z, Hong D, Lu P*, Wang YG*, Lin XF, Cascade Synthesis of Substituted 4-Amino-1,2,4-triazol-3-ones from Aldehyde Hydrazones and Azodicarboxylates, Tetrahedron 2010, 66(13), 2427-2432.
92. Hu BB, Wang YF, Chen XP, Zhao ZJ, Jiang ZT, Lu P*, Wang YG*, Synthesis and photophysical properties of tetrafluorophenyl-modified carbazole oligomers, Tetrahedron 2010, 66(38), 7583-7589.
93. Lu P, Wang YG* Strategies for Heterocyclic Synthesis via Cascade Reactions Based on Ketenimines, Synlett 2010, 165-173. (Account).
94. Wang, J.; He, Z. X.; Chen, X. P.; Song, W. Z.; Lu, P.*, Wang, Y. G.* Efficient Access to Polysubstituted Amidines, Benzimidazoles and Perimidines from Amides, Tetrahedron 2010, 66, 1208-1204.
95. Zhu YX, Wang SY, Wen S, Lu P*, Wang YG*, Copper-catalyzed cascade approach to 1,3-diazabicyclo[3.1.0]hex-3-enes from aziridines and ethyl diazoacetate, Tetrahedron Lett. 2010, 51(36), 4763-4766.
96. Hong D, Lin XF*, Zhu YX, Lei M, Wang YG*，Copper-Catalyzed Tandem Nucleophilic Ring-Opening/ Intramolecular Oxidative Amidation of N-Tosylaziridines and Hydrazones under Aerobic Conditions, Org. Lett. 2009, 11(24), 5678-5681.
97. Wang SY, Zhu YX, Wang YG*, Lu P*, Synthesis of Functionalized Indenes via Cascade Reaction of Aziridines and Propargyl Alcohols, Org. Lett. 2009, 11(12), 2615-2618.
98. 63. Lu W, Song WZ, Hong D, Lu P, Wang YG*, Copper-catalyzed one-pot synthesis of 2-methylidene-1,2,3,4-tetrahydropyrimidines, Adv. Synth. Catal. 2009, 351, 1768-1772.
99. Wang M, Xie MH, Wu CD*, Wang YG*, From one to three: a serine derivate manipulated homochiral metal-organic framework, Chem. Commun. 2009, 2396-2398.
100. Chen ZB, Hong D, Wang YG*, A Cascade Approach to Pyridines from 2-Azido-2, 4-dienoates and α-Diazocarbonyl Compounds, J. Org. Chem. 2009, 74(2), 903-905.
101. Chen ZB, Shou WG, Wang YG*, One-Pot Synthesis of 1,4-Diarylnaphthalenes via a Wittig-Horner Reaction/[4+2] Cycloaddition/Dehydrogenation Sequence, Synthesis 2009, 1075-1080.
102. She J, Jiang Z, Wang YG*, One-Pot Synthesis of Functionalized Benzimidazoles and 1H-Pyrimidines via Cascade Reactions of o-Aminoanilines or Naphthalene-1,8-diamine with Alkynes and p-Tolylsulfonyl Azide, Synlett 2009, (12), 2023-2027.
103. She J, Jiang Z, Wang YG*, Simple, efficient and recyclable catalytic system for performing copper-catalyzed C-S coupling of thiols with aryl iodides in PEG and PEG-H2O, Tetrahedron Lett. 2009, 50(5), 593-596.
104. Liu Y, Liu SL, Wang YG*, TEMPO-based Redox-sensitive Fluorescent Probes and Their Applications to Evaluating Intracellular Redox Status in Living Cells, Chem. Lett. 2009, 38(6), 588-589.
105. Chen XH, Chen XP, Zhao ZJ, Lu P*, Wang YG*, 2,4-Dicyano-3-diethylamino-9,9- diethylfluorene Based Blue Light-emitting Star-shaped Compounds: Synthesis and Properties, Chin. J. Chem. 2009, 27(5), 971-977.
106. Cui SL, Wang J, Wang YG*, Synthesis of Indoles via Domino Reaction of N-Aryl Amides and Ethyl Diazoacetate, J. Am. Chem. Soc. 2008, 130(41), 13526 - 13527.
107. Yang YY, Shou WG, Chen ZB, Hong D, Wang YG*, A Tandem Approach to Isoquinolines from 2-Azido-3-arylacrylates and a-Diazocarbonyl Compounds, J. Org. Chem. 2008, 73 (10), 3928-3930.
108. Yang YY, Shou WG, Hong D, Wang YG*, Selective Synthesis of 4-Alkylidene-b-lactams and N,N′-Diarylamidines from Azides and Aryloxyacetyl Chlorides via a Ketenimine-Participating One-Pot Cascade Process, J. Org. Chem. 2008, 73 (9), 3574-3577.
109. Cui SL, Wang J, Wang YG*, Copper-Catalyzed Multicomponent Reaction: Facile Access to Novel Phosphorous Amidines，Org. Lett. 2008, 10(6), 1267-1269.
110. Cui SL, Wang J, Wang YG*, Facile Access to Pyrazolines via Domino Reaction of the Huisgen Zwitterions with Aziridines, Org. Lett. 2008, 10 (1), 13-16.
111. Cui SL, Wang J, Wang YG*, Efficient Synthesis of 2-Imino-1,2- dihydroquinolines and 2-Imino-thiochromenes via Copper-catalyzed Domino Reaction, Tetrahedron 2008, 64, 487-492.
112. Hu RJ, Lei M, Xiong HS, Mu X, Wang YG*, Yin XF, Highly selective acylation of ferrocene using microfluidic chip reactor, Tetrahedron Lett. 2008, 49, 387-389.
113. Cui SL, Wang J, Wang YG*, Copper-Catalyzed Multicomponent Reaction: Facile Access to Functionalized 5-Arylidene-2-imino-3-pyrrolines, Org. Lett. 2007, 9 (24), 5023-5025.
114. Cui SL, Wang J, Lin XF, Wang YG*, Domino Reaction of 3-(2-Formylphenoxy)-propenoates and Amines: A Novel Synthesis of 1,4-Dihydropyridines from Salicaldehydes, Ethyl Propiolate and Amines, J. Org. Chem. 2007, 72 (20), 7779-7782.
115. Yang YY, Shou WG, Wang YG*, Tandem Coupling Reactions of Benzynes and 1,3-Diones: A Novel Synthesis of 2,2-diphenyl-1,3-Diones，Tetrahedron Lett. 2007, 48 (46), 8163-8165.
116. Du LH, Wang YG*, A rapid and efficient synthesis of benzimidazoles using hypervalent iodine as oxidant, Synthesis 2007, (5), 675-678.
117. Wang YG*, Cui SL, Lin XF, A Highly Selective Cascade Aprproach to Diverse Aromatic Ring Systems from Simple Aromatic Aldehydes and Propiolates，Org. Lett. 2006, 8(6), 1241-1244.
118. Cui SL, Lin XF, Wang YG*, Novel and efficient synthesis of iminocoumarins via copper-catalyzed multicomponent reaction, Org. Lett. 2006, 8(20), 4517-4520.
119. Shou WG, Yang YY, Wang YG*, Cascade approach to substituted 6-aryl-phenanthridines from aromatic aldehydes, anilines and benzenediazonium-2-carboxylate, J. Org. Chem. 2006, 71 (24), 9241-9243.
120. Ma C*, Ding HF, Wang YG, Novel Annulation Reactions of Aryl Methyl Ketenes with Zwitterions Derived from Dimethyl Acetylenedicarboxylate and N-Alkylimidazoles, Org. Lett. 2006, 8(14), 3133-3136.
121. Wang L, Zhang YH*, Liu LF, Wang YG*, Palladium-Catalyzed Homocoupling and Cross-Coupling Reactions of Aryl Halides in Poly(ethylene glycol), J. Org. Chem. 2006, 71 (3), 1284-1287.
122. Cui SL, Lin XF, Wang YG*, Cascade Reactions of Aromatic Aldehydes with Electron-Deficient Acetylenes: Regioselective Construction of Diverse Aromatic Ring Systems, Eur. J. Org. Chem. 2006, (22), 5174-5183.
123. Zhou FY, She J, Wang YG*, Synthesis of a benzyl-protected analog of arenarioside, a trisaccharide phenylpropanoid glycoside, Carbohydrate Res. 2006, 341, 2469-2477.
124. Yang YY, Shou WG, Wang YG*, Synthesis of beta-amino carbonyl compounds via a Zn(OTf)2-catalyzed cascade reaction of anilines with aromatic aldehydes and carbonyl compounds, Tetrahedron 2006, 62, 10079-10086.
125. Lei M, Hu RJ, Wang YG*, Mild and selective oxidation of alcohols to aldehydes and ketones using NaIO4/TEMPO/NaBr system under acidic conditions, Tetrahedron 2006, 62(38), 8928-8932.
126. Li SJ, Zhong JH, Wang YG*, Synthesis of new chiral N-heterocyclic carbenes from naturally occurring podophyllotoxin and their application to asymmetric allylic alkylation, Tetrahedron: Asymmetry 2006, 17(11), 1650-1654.
127. Huang JY, Li SJ, Wang YG*, TEMPO-linked metalloporphyrins as efficient catalysts for selective oxidation of alcohols and sulfides, Tetrahedron Lett. 2006, 47(32), 5637-5640.
128. Lin XF, Cui SL,Wang YG*, A highly efficient synthesis of 1,2,3,4-tetrahydroquinolines by molecular iodine-catalyzed domino reaction of anilines with cyclic enol ethers, Tetrahedron Lett. 2006, 47, 4509~4512.
129. Huang, HY; Lei, M; Wang, YG*, A novel and efficient ionic liquid supported synthesis of oligosaccharides, Tetrahedron Lett. 2006, 47, 3047-3050.
130. Lin, XF; Cui, SL; Wang, YG*, Molecular iodine-catalyzed one-pot synthesis of substituted quinolines from imines and aldehydes, Tetrahedron Lett. 2006, 47, 3127-3130.
131. Shou, WG; Yang, YY; Wang, YG*, An efficient synthesis of beta-amino esters via Zn(OTf)2-catalyzed Mannich-type reaction, Tetrahedron Lett. 2006, 47, 1845-1847.
132. Jian SZ, Yuan Q, Wang YG*, Diastereoselective synthesis of trans beta-lactams on soluble polymer support, Synthesis 2006, (11), 1829-1835.
133. Yuan Q, Jian SZ, Wang YG*, Enantioselective synthesis of beta-lactams using a chiral auxiliary, Synlett 2006, (7), 1113-1115.
134. Liu LF, Zhang YH*, Wang YG, Phosphine-free palladium acetate catalyzed Suzuki reaction in water, J. Org. Chem. 2005, 70 (15): 6122-6125.
135. Cui SL, Lin XF, Wang YG*, Parallel Synthesis of Strongly Fluorescent Polysubstituted 2,6-Dicyanoanilines via Microwave-promoted Multicomponent Reaction, J. Org. Chem. 2005, 70(7), 2866-2869.
136. Ding HF, Ma C*, Yang YW, Wang YG*, Unexpected Reaction of Dimethyl Acetylenedicarboxylate with in Situ Generated Arylketenes Catalyzed By 1-Methylimidazole, Org. Lett. 2005, 7(11), 2125-2127.
137. Luo CC, Zhang YH, Wang YG*, Palladium nanoparticles in poly(ethyleneglycol): the efficient and recyclable catalyst for Heck reaction, J. Mol. Catal. A: Chem. 2005, 229, 7–12.
138. Shou WG, Yang YY, Wang YG*, Liquid-phase Syntheses of 2, 3-Dihydro-4-pyridones and β-lactams from PEG-supported Aldehydes, Synthesis 2005, (4), 530-536.
139. Shou WG, Yang YY, Wang YG*, Parallel synthesis of strongly fluorescent tetraaryl-4,5-dihydro-1,2,4-triazoles via 1,3-dipolar cycloaddition on soluble polymer support, Synthesis 2005, (20), 3535-3540.
140. Jia SZ, Ma C, Wang YG*, An Efficient and Diastereoselective Synthesis of trans β-Lactams and β-Aminocarbonyl Compounds, Synthesis 2005, (5), 725-730.
141. Li SJ, Wang YG*, A novel and selective catalytic oxidation of hydrocarbons to ketones using chloramine-T/O-2/Fe(TPP)Cl system, Tetrahedron Lett. 2005，46 (46): 8013-8015.
142. Du LH, Zhang SJ, Wang YG*, Phenacyl esters as a new photocleavable linker in liquid-phase chemistry, Tetrahedron Lett. 2005, 46, 3399-3402.
143. Li WJ, Lin XF, Wang J, Li GU, Wang YG*, Palladium-catalyzed Michael addition of indoles to alpha,beta-unsaturated ketones in an ionic liquid, Synlett 2005, (13), 2003-2006.
144. Wang L, Zhang YH, Xie CS, Wang YG*, PEG-supported imidazolium chloride: A highly efficient and reusable reaction medium for the Heck reaction, Synlett 2005, (12), 1861-1864.
145. Xu G, Wang YG*, Microwave-assisted amination from aryl triflates without base and catalyst, Org. Lett. 2004, 6, 985-987.
146. Wang YG*, Wu XX, Jiang ZY, A mild and efficient selective tetrahydropyranylation of primary alcohols and deprotection of THP ethers of phenols and alcohols using PdCl2(CH3CN)2 as catalyst, Tetrahedron Lett. 2004, 45, 2973- 2976.
147. Cui SL, Jiang ZY, Wang YG*, A general and efficient protocol for the synthesis of biaryl ethers from aryl silyl ethers using Cs2CO3, Synlett 2004, 1829-1831.
148. Wang YG*, Lin XF, Cui SJ, An efficient protocol for the liquid-phase synthesis of furanoquinolines and pyranoquinolines, Synlett 2004, 1175-1178.
149. Wang YG*, Zhang J, Lin XF, et al. Parallel synthesis of pyrazolines on soluble polymer support, Synlett 2003, (10), 1467-1468.
150. Lin XF, Zhang J, Cui SL, Wang YG*, Poly(ethylene glycol) supported liquid-phase synthesis of 1,2,4-oxadiazolines，Synthesis 2003, (10), 1569-1573.
151. Shang YJ, Shou WG, Wang YG*, Synthesis of 1,2,4-oxadiazolines on soluble polymer support, Synlett 2003, (7), 1064-1066.
152. Lin XF, Zhang J, Wang YG*, Parallel synthesis of 4,5-dihydro-1,2,4- oxadiazoles using soluble polymer support, Tetrahedron Lett. 2003, 44 (21), 4113-4115.
153. Jiang ZY, Wang YG*, A mild, efficient and selective deprotection of t-butyldimethylsilyl-protected phenols using cesium carbonate, Tetrahedron Lett. 2003, 44 (19), 3859-3861.
154. Lin, XF; Cui, SL; Wang, YG, Rapid one-pot solid-phase synthesis of 1,2,4-oxadiazolines, CHEM. LETT. 2003, 32 (9), 842-843.
155. Jiang, ZY; Wang, YG, A mild, efficient and selective cleavage of aryl tert-butyldimethysilyl ethers using KOH in ethanol, CHEM. LETT. 2003, 32 (7), 568-569 .
156. Shang, YJ; Shou, WG; Wang, YG, Synthesis of 1,2,4-oxadiazolines on soluble polymer support, Synlett 2003, (7), 1064-1066.
157. Zhang, SJ; Dong, JQ; Wang, YG*, Synthesis and biological activities of novel seleno epi-daunomycin derivatives, Synth. Commun. 2003, 33 (11), 1891-1898.
158. Xu, H; Wang, YG*, A rapid and efficient Biginelli reaction catalyzed by zinc triflate, CHIN. J. CHEM. 2003, 21 (3), 327-331.
159. Xia, M; Wang, YG*, Polyethylene glycol supported chloro[1,3,5]triazine: A novel synthetic auxiliary for the liquid-phase synthesis of alkynyl benzamide derivatives, Synth. Commun. 2003, 33 (3), 403-408.
160. Shang, YJ; Wang, YG. One-pot synthesis of isoxazolines using soluble polymer-supported acrylate, CHIN. J. CHEM. 2003, 21 (1), 7-8.
161. Shang YJ, Wang YG*, Soluble polymer-supported synthesis of isoxazoles, Tetrahedron Lett. 2002, 43 (12), 2247-2249.
162. Xia M, Wang YG*, Soluble polymer-supported synthesis of Biginelli compounds, Tetrahedron Lett. 2002, 43 (43), 7703-7705.
163. Shang YJ, Wang YG*, Synthesis of isoxazolines and isoxazoles using poly(ethylene glycol) as support, Synthesis 2002, (12), 1663-1668.
164. Zhang SJ, Jia ZP, Wang YG*, Design, synthesis and antitumor activities of novel 7-arylseleno-7-deoxy-daunomycinone derivatives, Bioorganic & Medicinal Chem. 2002, 10(12), 3899-3904.
165. Zhang, SJ; Wang, YG, A facial synthesis of 7-selenodaunomycinone derivatives, J. CHEM. RES.-S 2001, (12), 520-521.
166. Lei, M; Ma, C; Wang, YG*, Polymer-supported 4-aminoformoyldiphenylammonium triflate (PS-AFDPAT): An efficient, recoverable and recyclable catalyst for esterification of carboxylic acids with equimolar amounts of alcohols, Chin. J. Chem. 2001, 19 (12), 1309-1311.
167. Ren, HJ; Wang, YG, A novel synthesis of beta-aryl-alpha,beta-unsaturated amides, Synth. Commun. 2001, 31 (8), 1201-1204.
168. Xu, SJ; Ma, C; Wang, YG; Chen, YZ, Synthesis of novel spin labeled analogues of N-(trifluoroacetyl)daunorubicin, Synth. Commun. 2000, 30 (13), 2375-2382.
169. Ma, C; Wang, YG; Chen, YZ, Synthesis and antitumor activities of spin labeled derivatives of daunorubicin and doxorubicin, Chem. J. Chin. Univ. 2000, 21 (6), 884-887.
170. Ma, C; Wang, YG; Shi, JF; Chen, YZ; Chen, YH, An efficient synthesis of N-trifluoroacetyl adriamycin-14-valerate (AD-32), Synth. Commun. 1999, 29 (20), 3581-3586.
171. Tao, L; Wang, YG; Ma, C; Zheng, B; Chen, YZ, Synthesis of novel 4 beta-(1,2,3-triazol-1-yl) podophyllotoxins as potential antitumor drugs, Synth. Commun. 1999, 29 (12), 2053-2059.
172. Wang YG, Pan JL, Shi JF, et al., New spin labelled analogues of podophyllotoxin as potential antitumor agents, Life Sci. 1997, 61 (5), 537-542.
173. Tian X, Wang YG, Yang MG, et al., Synthesis and antitumor activity spin labeled derivatives of podophyllotoxin, Life Sci. 1997, 60 (8), 511-517.
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发表于 2018-4-5 15:49:45
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